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Angelina Jolie has such large, lovely eyes and a truly engaging smile. I love it when people's smiles just light up their whole face.

Flashback to when Angelina Jolie appeared on MTV's TRL back in 2003! Check out the ultimate TRL time machine for pictures of your favorite stars in the '90s and early 2000s.

100+ TRL Moments That Will Bring You Right Back to the Early 2000s

Angelina Jolie flashed a big smile during her TRL appearance in

Brad Pitt and Angelina Jolie shared a laugh with a colleague during at the Screen Actors Guild Awards, 2009.

Brad Pitt and Angelina Jolie shared a laugh with a colleague during at the Screen Actors Guild Awards,

Angelina Jolie Looking Beautiful Women your email address please click here I will never forget how you can see there is no Brad Pitt in my eye's you & yours 6 pk yes I Truly Admire you Dear Mother Angie's your an Angie in my Hart and eyes note that OK Your

Angelina Jolie Looking Beautiful Women your email address please click here I will never forget how you can see there is no Brad Pitt in my eye's you & yours 6 pk yes I Truly Admire you Dear Mother Angie's your an Angie in my Hart and eyes note that OK Your

LOVE the gray color...and gorgeous Angie is wearing it and the dress (St. John's) is so beautifully intricate...did i mention it's gray?

Brad Pitt and Angelina Jolie: The Way They Were

Angelina Jolie & Brad Pitt at the 2007 Golden Globes (Angelina is wearing a St John Couture gown)

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Angelina Jolie Is Named Honorary Dame By Queen Elizabeth

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